Pr magnetism and its interplay with the Fe spin density wave in PrFeAsO

We have studied the magnetism of the Pr3+ ions in PrFeAsO_1-xF_x (x = 0; 0.15) and its interaction with the Fe magnetic order (for x = 0). Specific heat data confirm the presence of a first excited crystal electric field (CEF) level around 3.5 meV in the undoped compound PrFeAsO. This finding is in agreement with recent neutron scattering experiments. The doped compound is found to have a much lower first CEF splitting of about 2.0 meV. The Pr ordering in PrFeAsO gives rise to large anomalies in the specific heat and the thermal expansion coefficient. In addition, a field-induced transition is found at low temperatures that is most pronounced for the magnetostriction coefficient. This transition, which is absent in the doped compound, is attributed to a reversal of the Fe spin canting as the antiferromagnetic Pr order is destroyed by the external magnetic field.Comment: 8 pages, 6 figure

Interaction-induced singular Fermi surface in a high-temperature oxypnictide superconductor

In the family of iron-based superconductors, LaFeAsO-type materials possess the simplest electronic structure due to their pronounced two-dimensionality. And yet they host superconductivity with the highest transition temperature Tc=55K. Early theoretical predictions of their electronic structure revealed multiple large circular portions of the Fermi surface with a very good geometrical overlap (nesting), believed to enhance the pairing interaction and thus superconductivity. The prevalence of such large circular features in the Fermi surface has since been associated with many other iron-based compounds and has grown to be generally accepted in the field. In this work we show that a prototypical compound of the 1111-type, SmFe0.92Co0.08AsO, is at odds with this description and possesses a distinctly different Fermi surface, which consists of two singular constructs formed by the edges of several bands, pulled to the Fermi level from the depths of the theoretically predicted band structure by strong electronic interactions. Such singularities dramatically affect the low-energy electronic properties of the material, including superconductivity. We further argue that occurrence of these singularities correlates with the maximum superconducting transition temperature attainable in each material class over the entire family of iron-based superconductors.Comment: Open access article available online at http://www.nature.com/srep/2015/150521/srep10392/full/srep10392.htm

Local magnetic anisotropy in BaFe2_2As2_2: a polarized inelastic neutron scattering study

The anisotropy of the magnetic excitations in BaFe$_2$As$_2$ was studied by polarized inelastic neutron scattering which allows one to separate the components of the magnetic response. Despite the in-plane orientation of the static ordered moment we find the in-plane polarized magnons to exhibit a larger gap than the out-of-plane polarized ones indicating very strong single-ion anisotropy within the layers. It costs more energy to rotate a spin within the orthorhombic {\it a-b} plane than rotating it perpendicular to the FeAs layers.Comment: 4 pages, 4 figure

Surface properties of SmB6 from x-ray photoelectron spectroscopy

We have investigated the properties of cleaved SmB$_6$ single crystals by x-ray photoelectron spectroscopy. At low temperatures and freshly cleaved samples a surface core level shift is observed which vanishes when the temperature is increased. A Sm valence between 2.5 - 2.6 is derived from the relative intensities of the Sm$^{2+}$ and Sm$^{3+}$ multiplets. The B/Sm intensity ratio obtained from the core levels is always larger than the stoichiometric value. Possible reasons for this deviation are discussed. The B $1s$ signal shows an unexpected complexity: an anomalous low energy component appears with increasing temperature and is assigned to the formation of a suboxide at the surface. While several interesting intrinsic and extrinsic properties of the SmB$_6$ surface are elucidated in this manuscript no clear indication of a trivial mechanism for the prominent surface conductivity is found

Ballistic heat transport of quantum spin excitations as seen in SrCuO2

Fundamental conservation laws predict ballistic, i.e., dissipationless transport behaviour in one-dimensional quantum magnets. Experimental evidence, however, for such anomalous transport has been lacking ever since. Here we provide experimental evidence for ballistic heat transport in a S=1/2 Heisenberg chain. In particular, we investigate high purity samples of the chain cuprate SrCuO2 and observe a huge magnetic heat conductivity $\kappa_{mag}$. An extremely large spinon mean free path of more than a micrometer demonstrates that $\kappa_{mag}$ is only limited by extrinsic scattering processes which is a clear signature of ballistic transport in the underlying spin model

High-temperature superconductivity from fine-tuning of Fermi-surface singularities in iron oxypnictides

In the family of the iron-based superconductors, the $RE$FeAsO-type compounds (with $RE$ being a rare-earth metal) exhibit the highest bulk superconducting transition temperatures ($T_{\mathrm{c}}$) up to $55\ \textrm{K}$ and thus hold the key to the elusive pairing mechanism. Recently, it has been demonstrated that the intrinsic electronic structure of SmFe$_{0.92}$Co$_{0.08}$AsO ($T_{\mathrm{c}}=18\ \textrm{K}$) is highly nontrivial and consists of multiple band-edge singularities in close proximity to the Fermi level. However, it remains unclear whether these singularities are generic to the $RE$FeAsO-type materials and if so, whether their exact topology is responsible for the aforementioned record $T_{\mathrm{c}}$. In this work, we use angle-resolved photoemission spectroscopy (ARPES) to investigate the inherent electronic structure of the NdFeAsO$_{0.6}$F$_{0.4}$ compound with a twice higher $T_{\mathrm{c}}=38\ \textrm{K}$. We find a similarly singular Fermi surface and further demonstrate that the dramatic enhancement of superconductivity in this compound correlates closely with the fine-tuning of one of the band-edge singularities to within a fraction of the superconducting energy gap $\Delta$ below the Fermi level. Our results provide compelling evidence that the band-structure singularities near the Fermi level in the iron-based superconductors must be explicitly accounted for in any attempt to understand the mechanism of superconducting pairing in these materials.Comment: Open access article available online at http://www.nature.com/articles/srep1827

NMR Evidence for Charge Inhomogeneity in Stripe Ordered La_{1.8-x}Eu_{0.2}Sr_{x}CuO_4

We report ^{17}O Nuclear Magnetic Resonance (NMR) results in the stripe ordered La_{1.8-x}Eu_{0.2}Sr_{x}CuO_4 system. Below a temperature T_q ~ 80K, the local electric field gradient (EFG) and the absolute intensity of the NMR signal of the planar O site exhibit a dramatic decrease. We interpret these results as microscopic evidence for a spatially inhomogeneous charge distribution, where the NMR signal from O sites in the domain walls of the spin density modulation are wiped out due to large hyperfine fields, and the remaining signal arises from the intervening Mott insulating regions.Comment: 4 pages, to appear in Phys. Rev. Let

Magnetisation of hole-doped CuO2 spin chains in Sr14-xCaxCu24O41

We report on magnetisation measurements of Sr14-xCaxCu24O41, with 0 <= x <= 12, in magnetic fields up to 16 T. The low temperature magnetic response of the CuO2 spin chains changes strongly upon doping. For x = 0, the ground state with nearly independent dimers is confirmed. Reduction of the number of holes in the chains through Ca-doping leads to an additional contribution to the magnetisation, which depends linearly on the magnetic field. Remarkably, the slope of this linear contribution increases with the Ca content. We argue that antiferromagnetic spin chains do not account for this behaviour but that the hole dynamics might be involved.Comment: In v2, spelling of author names has been change

Magnetization reversal and local switching fields of ferromagnetic Co/Pd microtubes with radial magnetization

Three-dimensional nanomagnetism is a rapidly growing field of research covering both noncollinear spin textures and curved magnetic geometries including microtubular structures. We spatially resolve the field-induced magnetization reversal of free-standing ferromagnetic microtubes utilizing multifrequency magnetic force microscopy (MFM). The microtubes are composed of Co/Pd multilayer films with perpendicular magnetic anisotropy that translates to an anisotropy with radial easy axis upon rolling-up. Simultaneously mapping the topography and the perpendicular magnetostatic force derivative, the relation between surface angle and local magnetization configuration is evaluated for a large number of locations with slopes exceeding 45 degrees. The angle-dependence of the switching field is concurrent with the Kondorsky model, i.e., the rolled-up nanomembrane behaves like a planar magnetic film with perpendicular anisotropy and a pinning dominated magnetization reversal. Additionally, we discuss methodological challenges when detecting magnetostatic force derivatives near steep surfaces